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Thermal radiative properties of metamaterials and other nanostructured materials: A review

Ceji FU, Zhuomin M. ZHANG

《能源前沿（英文）》 2009年 第3卷 第1期   页码 11-26 doi: 10.1007/s11708-009-0009-x

摘要： The ability to manufacture, control, and manipulate structures at extremely small scales is the hallmark of modern technologies, including microelectronics, MEMS/NEMS, and nano-biotechnology. Along with the advancement of microfabrication technology, more and more investigations have been performed in recent years to understand the influence of microstructures on radiative properties. The key to the enhancement of performance is through the modification of the reflection and transmission properties of electromagnetic waves and thermal emission spectra using one-, two-, or three-dimensional micro/nanostructures. This review focuses on recent developments in metamaterials–manmade materials with exotic optical properties, and other nanostructured materials, such as gratings and photonic crystals, for application in radiative energy transfer and energy conversion systems.

关键词： metamaterial     nanostructured material     thermal radiative property     radiative energy transfer    

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高性能纳米贝氏体轴承用钢发展与展望 Review

张福成, 杨志南

《工程（英文）》 2019年 第5卷 第2期   页码 319-328 doi: 10.1016/j.eng.2018.11.024

摘要：

轴承是几乎所有机械设备中最关键的零部件，能确保设备平稳运行，这对于高端装备尤为重要，如高速铁路客车和盾构机械等。随着技术的快速发展，对轴承质量的要求不断提高。轴承的制造水平直接反映一个国家钢铁冶金以及机械制造的水平。轴承钢的性能是决定轴承质量的关键因素。因此，开发更优异性能的轴承钢是材料研究领域与机械制造行业所共同追求的目标。国内外著名的轴承制造企业竞相开发新型轴承用钢。纳米贝氏体轴承钢是一类新开发的轴承钢，不仅具有高的强韧性，同时也表现出优异的耐磨性与抗滚动接触疲劳性能。近年来，中国学者在纳米贝氏体轴承钢方面的研究成果显著推动了这一领域的发展。在中国，纳米贝氏体轴承钢最先被用来制造大功率风电主轴轴承及其他重载轴承，表现出了优异的性能。因此，纳米贝氏体轴承钢和相关热处理技术首次被纳入国家标准和行业标准中。轴承行业认为纳米贝氏体轴承钢的开发具有划时代的意义，并称这种轴承为“第二代贝氏体轴承”。本文详细综述了纳米贝氏体轴承钢的发展，包括其优点和不足，并提出了下一步的研究方向。

关键词： 轴承钢     纳米贝氏体     发展     应用     展望    

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Leidenfrost drops on micro/nanostructured surfaces

Vishal TALARI, Prakhar BEHAR, Yi LU, Evan HARYADI, Dong LIU

《能源前沿（英文）》 2018年 第12卷 第1期   页码 22-42 doi: 10.1007/s11708-018-0541-7

摘要： In the Leidenfrost state, the liquid drop is levitated above a hot solid surface by a vapor layer generated via evaporation from the drop. The vapor layer thermally insulates the drop from the heating surface, causing deteriorated heat transfer in a myriad of important engineering applications. Thus, it is highly desirable to suppress the Leidenfrost effect and elevate the Leidenfrost temperature. This paper presents a comprehensive review of recent literature concerning the Leidenfrost drops on micro/nanostructured surfaces with an emphasis on the enhancement of the Leidenfrost temperature. The basic physical processes of the Leidenfrost effect and the key characteristics of the Leidenfrost drops were first introduced. Then, the major findings of the influence of various micro/nanoscale surface structures on the Leidenfrost temperature were presented in detail, and the underlying enhancement mechanism for each specific surface topology was also discussed. It was concluded that multiscale hierarchical surfaces hold the best promise to significantly boost the Leidenfrost temperature by combining the advantages of both micro- and nanoscale structures.

关键词： Leidenfrost drop     Leidenfrost temperature     heat transfer enhancement     micro/nanostructured surfaces    

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Preface to special issue on “Engineering Nanostructured Materials for Advanced Energy and Environmental

《化学科学与工程前沿（英文）》 2023年 第17卷 第11期   页码 1621-1622 doi: 10.1007/s11705-023-2365-1

摘要： Preface to special issue on “Engineering Nanostructured Materials for Advanced Energy and Environmental Catalysis”
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New nanostructured sorbents for desulfurization of natural gas

Lifeng WANG, Ralph T. YANG

《化学科学与工程前沿（英文）》 2014年 第8卷 第1期   页码 8-19 doi: 10.1007/s11705-014-1411-4

摘要： Desulfurization of natural gas is achieved commercially by absorption with liquid amine solutions. Adsorption technology could potentially replace the solvent extraction process, particularly for the emerging shale gas wells with production rates that are generally lower than that from the large conventional reservoirs, if a superior adsorbent (sorbent) is developed. In this review, we focus our discussion on three types of sorbents: metal-oxide based sorbents, Cu/Ag-based and other commercial sorbents, and amine-grafted silicas. The advantages and disadvantages of each type are analyzed. Possible approaches for future developments to further improve these sorbents are suggested, particularly for the most promising amine-grafted silicas.

关键词： desulfurization     natural gas desulfurization     hydrogen sulfide sorbent     amine-silica sorbent    

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Structural engineering of transition metal-based nanostructured electrocatalysts for efficient water

Yueqing Wang, Jintao Zhang

《化学科学与工程前沿（英文）》 2018年 第12卷 第4期   页码 838-854 doi: 10.1007/s11705-018-1746-3

摘要： Water splitting is a highly promising approach for the generation of sustainable, clean hydrogen energy. Tremendous efforts have been devoted to exploring highly efficient and abundant metal oxide electrocatalysts for oxygen evolution and hydrogen evolution reactions to lower the energy consumption in water splitting. In this review, we summarize the recent advances on the development of metal oxide electrocatalysts with special emphasis on the structural engineering of nanostructures from particle size, composition, crystalline facet, hybrid structure as well as the conductive supports. The special strategies relay on the transformation from the metal organic framework and ion exchange reactions for the preparation of novel metal oxide nanostructures with boosting the catalytic activities are also discussed. The fascinating methods would pave the way for rational design of advanced electrocatalysts for efficient water splitting.

关键词： water splitting     structure engineering     metal organic framework     ion exchange     synergistic effect     hybrid structure     conductive supports    

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Modeling nanostructured catalyst layer in PEMFC and catalyst utilization

Jiejing ZHANG, Pengzhen CAO, Li XU, Yuxin WANG

《化学科学与工程前沿（英文）》 2011年 第5卷 第3期   页码 297-302 doi: 10.1007/s11705-011-1201-1

摘要： A lattice model of the nanoscaled catalyst layer structure in proton exchange membrane fuel cells (PEMFC) was established by Monte Carlo method. The model takes into account all the four components in a typical PEMFC catalyst layer: platinum (Pt), carbon, ionomer and pore. The elemental voxels in the lattice were set fine enough so that each average sized Pt particulate in Pt/C catalyst can be represented. Catalyst utilization in the modeled catalyst layer was calculated by counting up the number of facets of Pt voxels where “three phase contact” are met. The effects of some factors, including porosity, ionomer content, Pt/C particle size and Pt weight percentage in the Pt/C catalyst, on catalyst utilization were investigated and discussed.

关键词： catalyst layer     PEM fuel cell     lattice model     Monte Carlo method     catalyst utilization    

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Structural and optical properties of nanostructured copper sulfide semiconductor synthesized in an industrial

Marcela Achimovičová, Erika Dutková, Erika Tóthová, Zdenka Bujňáková, Jaroslav Briančin, Satoshi Kitazono

《化学科学与工程前沿（英文）》 2019年 第13卷 第1期   页码 164-170 doi: 10.1007/s11705-018-1755-2

摘要：

Chalcogenide nanostructured semiconductor, copper sulfide (CuS) was prepared from copper and sulfur powders in stoichiometric ratio by a simple, fast, and convenient one-step mechanochemical synthesis after 40 min of milling in an industrial eccentric vibratory mill. The kinetics of the mechanochemical synthesis and the influence of the physical properties of two Cu powder precursor types on the kinetics were studied. The crystal structure, physical properties, and morphology of the product were characterized by X-ray diffraction (XRD), the specific surface area measurements, particle size distribution and scanning electron microscopy. The XRD analysis confirmed the hexagonal crystal structure of the product-CuS (covellite) with the average size of the crystallites 11 nm. The scanning electron microscopy analysis has revealed that the agglomerated grains have a plate-like structure composed of CuS nanoparticles. The thermal analysis was performed to investigate the thermal stability of the mechanochemically synthesized CuS. The optical properties were studied using UV-Vis and photoluminescence spectroscopy. The determined optical band gap energy 1.80 eV responds to the value of the bulk CuS, because of agglomerated nanoparticles. In addition, a mechanism of CuS mechanochemical reaction was proposed, and the verification of CuS commercial production was performed.

关键词： copper sulfide     industrial mechanochemical synthesis     thermal analysis     optical properties    

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3D Network nanostructured NiCoP nanosheets supported on N-doped carbon coated Ni foam as a highly active

Miaomiao Tong, Lei Wang, Peng Yu, Xu Liu, Honggang Fu

《化学科学与工程前沿（英文）》 2018年 第12卷 第3期   页码 417-424 doi: 10.1007/s11705-018-1711-1

摘要：

A highly active bi-functional electrocatalyst towards both hydrogen and oxygen evolution reactions is critical for the water splitting. Herein, a self-supported electrode composed of 3D network nanostructured NiCoP nanosheets grown on N-doped carbon coated Ni foam (NiCoP/NF@NC) has been synthesized by a hydrothermal route and a subsequent phosphorization process. As a bifunctional electrocatalyst, the NiCoP/NF@NC electrode needs overpotentials of 31.8 mV for hydrogen evolution reaction and 308.2 mV for oxygen evolution reaction to achieve the current density of 10 mA·cm−2 in 1 mol·L−1 KOH electrolyte. This is much better than the corresponding monometal catalysts of CoP/NF@NC and NiP/NF@NC owing to the synergistic effect. NiCoP/NF@NC also exhibits low Tafel slope, and excellent long-term stability, which are comparable to the commercial noble catalysts of Pt/C and RuO2.

关键词： bimetallic phosphides     N-doped carbon     self-support     hydrogen evolution     oxygen evolution    

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Liquid metal material genome: Initiation of a new research track towards discovery of advanced energy

Lei WANG, Jing LIU

《能源前沿（英文）》 2013年 第7卷 第3期   页码 317-332 doi: 10.1007/s11708-013-0271-9

摘要： As the basis of modern industry, the roles materials play are becoming increasingly vital in this day and age. With many superior physical properties over conventional fluids, the low melting point liquid metal material, especially room-temperature liquid metal, is recently found to be uniquely useful in a wide variety of emerging areas from energy, electronics to medical sciences. However, with the coming enormous utilization of such materials, serious issues also arise which urgently need to be addressed. A biggest concern to impede the large scale application of room-temperature liquid metal technologies is that there is currently a strong shortage of the materials and species available to meet the tough requirements such as cost, melting point, electrical and thermal conductivity, etc. Inspired by the Material Genome Initiative as issued in 2011 by the United States of America, a more specific and focused project initiative was proposed in this paper—the liquid metal material genome aimed to discover advanced new functional alloys with low melting point so as to fulfill various increasing needs. The basic schemes and road map for this new research program, which is expected to have a worldwide significance, were outlined. The theoretical strategies and experimental methods in the research and development of liquid metal material genome were introduced. Particularly, the calculation of phase diagram (CALPHAD) approach as a highly effective way for material design was discussed. Further, the first-principles (FP) calculation was suggested to combine with the statistical thermodynamics to calculate the thermodynamic functions so as to enrich the CALPHAD database of liquid metals. When the experimental data are too scarce to perform a regular treatment, the combination of FP calculation, cluster variation method (CVM) or molecular dynamics (MD), and CALPHAD, referred to as the mixed FP-CVM-CALPHAD method can be a promising way to solve the problem. Except for the theoretical strategies, several parallel processing experimental methods were also analyzed, which can help improve the efficiency of finding new liquid metal materials and reducing the cost. The liquid metal material genome proposal as initiated in this paper will accelerate the process of finding and utilization of new functional materials.

关键词： liquid metal material genome     energy material     material discovery     advanced material     room-temperature liquid alloy     thermodynamics     phase diagram    

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Robust topology optimization of multi-material lattice structures under material and load uncertainties

Yu-Chin CHAN, Kohei SHINTANI, Wei CHEN

《机械工程前沿（英文）》 2019年 第14卷 第2期   页码 141-152 doi: 10.1007/s11465-019-0531-4

摘要： Enabled by advancements in multi-material additive manufacturing, lightweight lattice structures consisting of networks of periodic unit cells have gained popularity due to their extraordinary performance and wide array of functions. This work proposes a density-based robust topology optimization method for meso- or macro-scale multi-material lattice structures under any combination of material and load uncertainties. The method utilizes a new generalized material interpolation scheme for an arbitrary number of materials, and employs univariate dimension reduction and Gauss-type quadrature to quantify and propagate uncertainty. By formulating the objective function as a weighted sum of the mean and standard deviation of compliance, the tradeoff between optimality and robustness can be studied and controlled. Examples of a cantilever beam lattice structure under various material and load uncertainty cases exhibit the efficiency and flexibility of the approach. The accuracy of univariate dimension reduction is validated by comparing the results to the Monte Carlo approach.

关键词： robust topology optimization     lattice structures     multi-material     material uncertainty     load uncertainty     univariate dimension reduction    

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工程材料研究中科学问题的思考

于翘

《中国工程科学》 1999年 第1卷 第3期   页码 1-4

摘要：

在不少场合下，航天用工程材料处在极端条件下工作，这就对材料提出许多特殊的要求，虽然国内外有一定的研究积累，但对更精确的模型和符合特定材料的损伤的状态方程，有待深一步研究。如高级弹头再入时气动加热和粒子云侵蚀以及两者耦合效应引起弹头防护材料增大后退量的问题；空中垃圾和微流星的高速碰撞对航天器的威胁；特别是核爆和激光武器对材料的损伤和破坏，实质上是辐射引起的热击波层裂破坏，这些都属于超高速碰撞对材料的响应问题。天线罩材料、吸波材料、红外隐身材料、电磁屏蔽材料都是具有不同波长电磁波的电磁功能材料，它们对固体介质的穿透、吸收、反射等会产生响应，不同的电磁功能材料，其宏观性能的物理参量不同，但有几个参量是通用的，如介电常数、磁导率和损耗角正切，搞清这些参量与材料微观结构的关系，可以为材料设计和材料创新提供科学依据。

关键词： 天线罩材料     吸波材料     红外隐身材料     电磁兼容材料    

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Nanostructured hollow spheres of hydroxyapatite: preparation and potential application in drug delivery

Xiaojing ZHANG, Weixin ZHANG, Zeheng YANG, Zhao ZHANG

《化学科学与工程前沿（英文）》 2012年 第6卷 第3期   页码 246-252 doi: 10.1007/s11705-012-1299-9

摘要： A solvothermal method has been successfully used to prepare nanostructured hydroxyapatite (HA) hollow spheres with average diameters of about 500 nm and shell thicknesses of about 100 nm in a glycerin/water mixed solvent. Transmission electron microscopy (TEM) and field-emission scanning electron microscopy (FESEM) images show that the shells of the HA hollow spheres are actually composed of nanosheets with thicknesses of about 10 nm. By tuning the glycerin/water volume ratio, two other kinds of HA solid spheres with average diameters of about 6 or 20 μm were assembled from nanoflakes. The properties of the different kinds of spheres as drug delivery carriers were evaluated. Ibuprofen (IBU) was chosen as the model drug to load into the HA samples. The nanostructured HA samples showed a slow and sustained release of IBU. The HA hollow spheres exhibited a higher drug loading capacity and more favorable release properties than the HA solid spheres and thus are very promising for controlled drug release applications.

关键词： hydroxyapatite     hollow spheres     synthesis     drug release    

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A novel approach to minimizing material loss for computer numerical control flank-regrinding of worn

《机械工程前沿（英文）》 2023年 第18卷 第3期 doi: 10.1007/s11465-023-0757-z

摘要： Flanks of end mills are prone to wear in a long machining process. Regrinding is widely used in workshops to restore the flank to an original-like state. However, the traditional method involves material waste by trial and error and dramatically decreases the potential regrinding. Moreover, over-cut would happen to the flutes of worn cutters in the regrinding processes because of improper wheel path. This study presented a new approach to planning the wheel path for regrinding worn end mills to minimize material loss and recover the over-cut. In planning, a scaling method was developed to determine the maximum size of the new cutter according to the similarity of cutter shapes before and after regrinding. Then, the wheel path is first generated by envelope theory to regrind the worn area with a four-axis computer numerical control grinder according to the new size of cutters. Moreover, a second regrinding strategy is applied to recover the flute shape over-cut in the first grinding. Finally, the proposed method is verified by an experiment. Results showed that the proposed approach could save 25% of cutter material compared with the traditional method and ensure at least three regrinding times. This work effectively provides a general regrinding solution for the worn flank with maximum material-saving and regrinding period.

关键词： flank-regrinding     worn end mill     wheel position and orientation     material loss     over-cut    

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A MATLAB code for the material-field series-expansion topology optimization method

《机械工程前沿（英文）》 2021年 第16卷 第3期   页码 607-622 doi: 10.1007/s11465-021-0637-3

摘要： This paper presents a MATLAB implementation of the material-field series-expansion (MFSE) topo-logy optimization method. The MFSE method uses a bounded material field with specified spatial correlation to represent the structural topology. With the series-expansion method for bounded fields, this material field is described with the characteristic base functions and the corresponding coefficients. Compared with the conventional density-based method, the MFSE method decouples the topological description and the finite element discretization, and greatly reduces the number of design variables after dimensionality reduction. Other features of this method include inherent control on structural topological complexity, crisp structural boundary description, mesh independence, and being free from the checkerboard pattern. With the focus on the implementation of the MFSE method, the present MATLAB code uses the maximum stiffness optimization problems solved with a gradient-based optimizer as examples. The MATLAB code consists of three parts, namely, the main program and two subroutines (one for aggregating the optimization constraints and the other about the method of moving asymptotes optimizer). The implementation of the code and its extensions to topology optimization problems with multiple load cases and passive elements are discussed in detail. The code is intended for researchers who are interested in this method and want to get started with it quickly. It can also be used as a basis for handling complex engineering optimization problems by combining the MFSE topology optimization method with non-gradient optimization algorithms without sensitivity information because only a few design variables are required to describe relatively complex structural topology and smooth structural boundaries using the MFSE method.

关键词： MATLAB implementation     topology optimization     material-field series-expansion method     bounded material field     dimensionality reduction    

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标题 作者 时间 类型 操作

Thermal radiative properties of metamaterials and other nanostructured materials: A review

Ceji FU, Zhuomin M. ZHANG

期刊论文

高性能纳米贝氏体轴承用钢发展与展望

张福成, 杨志南

期刊论文

Leidenfrost drops on micro/nanostructured surfaces

Vishal TALARI, Prakhar BEHAR, Yi LU, Evan HARYADI, Dong LIU

期刊论文

Preface to special issue on “Engineering Nanostructured Materials for Advanced Energy and Environmental

期刊论文

New nanostructured sorbents for desulfurization of natural gas

Lifeng WANG, Ralph T. YANG

期刊论文

Structural engineering of transition metal-based nanostructured electrocatalysts for efficient water

Yueqing Wang, Jintao Zhang

期刊论文

Modeling nanostructured catalyst layer in PEMFC and catalyst utilization

Jiejing ZHANG, Pengzhen CAO, Li XU, Yuxin WANG

期刊论文

Structural and optical properties of nanostructured copper sulfide semiconductor synthesized in an industrial

Marcela Achimovičová, Erika Dutková, Erika Tóthová, Zdenka Bujňáková, Jaroslav Briančin, Satoshi Kitazono

期刊论文

3D Network nanostructured NiCoP nanosheets supported on N-doped carbon coated Ni foam as a highly active

Miaomiao Tong, Lei Wang, Peng Yu, Xu Liu, Honggang Fu

期刊论文

Liquid metal material genome: Initiation of a new research track towards discovery of advanced energy

Lei WANG, Jing LIU

期刊论文

Robust topology optimization of multi-material lattice structures under material and load uncertainties

Yu-Chin CHAN, Kohei SHINTANI, Wei CHEN

期刊论文

工程材料研究中科学问题的思考

于翘

期刊论文

Nanostructured hollow spheres of hydroxyapatite: preparation and potential application in drug delivery

Xiaojing ZHANG, Weixin ZHANG, Zeheng YANG, Zhao ZHANG

期刊论文

A novel approach to minimizing material loss for computer numerical control flank-regrinding of worn

期刊论文

A MATLAB code for the material-field series-expansion topology optimization method

期刊论文